congratulation to Our new paper in Journal of Thin solid films
Thermoplasmonic enhanced detection efficiency by gold nanoparticles/ chlorophyll heterojunction on silicon nanowires
S. Valimohammadi, S. M. Hamidi and L. Rajaee
https://doi.org/10.1016/j.tsf.2025.140837
Abstract:
This study presents the development of a ternary heterojunction nanostructure for visible-light detection at 532 nm. Silicon nanowires (SiNWs) were grown using the metal-assisted chemical etching (MACE) method. The structure incorporates gold nanoparticles (Au NPs), synthesized via laser ablation (a fixed amount of S0: 1500 µL), which were combined with varying concentrations of chlorophyll-a (Chl-a) (S1: 1000 µL, S2: 1500 µL, S3: 2000 µL). Characterization techniques included SEM and AFM to confirm SiNWs morphology, UV-Vis spectroscopy to examine the optical properties of the Au/Chl-a combination, and current-voltage (I-V) measurements to evaluate the enhanced photodetector performance. Key findings demonstrated that plasmon-exciton dipole interactions effectively increase electron-hole pair separation via the formation of plexcitons. Furthermore, thermoplasmonic heating raised the temperature of the optimal sample (SiNWs@S2) to 51.6°C (compared to the baseline SiNWs@S0 temperature of 40.7°C), representing a 26.78% improvement. This system shows promising potential for high-performance optical sensing applications.

Figure 2: (a-c) Cross sectional scanning electron microscopy (SEM) micrographs of SiNWs fabricated at 30 min etching time in HF (40%)/AgNO3 (0.1 M)/H2O2(30%) solutions having a volume ratio of: 16:5:60 (top row),(d) 2D AFM image of SiNW,(e)Height profile and slope (f) I-V curve of P-type silicon wafers and SiNW at different voltages.







